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Chem. BeE 100, 228 (1967). , Renk, I. : Chem. Ber. 100, 228 (1967). - - C h e m . Ber. 104, 110(1971). Tschugaeff, L. : J. Prakt. Chem. 75, 153 (1907). : J. Prakt. Chem. 124, 133 (1930). : Acta Cryst. 22, 468 (1967). : Introduction to Ligand Field Theory. New York: McGraw-Hill 1962. 128) lngraham, L. : Acta Chem. Scand. 20, 283 (1966). : J. Chem. Phys. 23, 1833, 1841 (1955). , Kamakura, Japan Contents I. I n t r o d u c t i o n . . . . . . . . . . . II. a-Bond F o r m a t i o n . .

5. F o r m a t i o n o f Metal Carbonylate Anions from Metal Carbonyls and Their Reactions . . . . . . . . . III. Insertion Reactions . . . . . . . . . IV. Liberation of Organic C o m p o u n d s from the a-Complexes V. Cyclization Reaction and Related Reactions 43 43 50 54 56 59 64 70 . . . . . 74 . . . . . . . . . 80 . . . . . . . . . . . 81 VI. Concluding Remarks VII. References .... 42 41 J. Tsuji I. Introduction The art of organic synthesis has been enriched by the development of new methods: remarkable advances have been made in the last 15 years by the use of transition metal complexes.

21, 258 (1953). : Tetrahedron Letters 1971, 541;Tetrahedron 27, 4609 (I 971). : Angew. Chem. 77, 1097 (1965). Ashe, A. : Tetrahedron Letters 1968, 359. : Tetrahedron Letters 1964, 1923. Coulson, C. : Proc. Roy. Soc. (London) A 164, 383 (1938). Frost, A. : J. Chem. Phys. 21, 572 (1953). Coulson, C. , Longuet-Higgins, H. : Proc. Roy. Soc. (London) A 191, 39 (1947); A 193, 447 (1948). : HMO-Hiickel Molecular Orbitals. Berlin-Heidelberg-New York: Springer 1966. : Chem. BeE 100, 228 (1967). , Renk, I.

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